I think I may have solved it. I noticed that in the collections on the desktop that the iPhone Photos collection only listed about 200 photos. I checked my iPhone, and the same collection had 900+ photos. Suddenly the number on the desktop started going down! My guess is that it was trying to sync the collections in order from top to bottom. Since the iPhone app wasn't open, it was stuck waiting for the iPhone to finish syncing TO the desktop. I'm hoping that once the iPhone finishes uploading that the desktop collections will start syncing down to the mobile devices. I'll report back soon.
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